• 中文核心期刊
  • 中国科技核心期刊
  • CSCD
  • ISSN 1007-6336
  • CN 21-1168/X
HUANG Ya-nan, WU Meng-meng, XIAO Zhi. Source and time series of 239+240Pu in marine corals[J]. Chinese Journal of MARINE ENVIRONMENTAL SCIENCE, 2022, 41(1): 65-73. DOI: 10.12111/j.mes.20200172
Citation: HUANG Ya-nan, WU Meng-meng, XIAO Zhi. Source and time series of 239+240Pu in marine corals[J]. Chinese Journal of MARINE ENVIRONMENTAL SCIENCE, 2022, 41(1): 65-73. DOI: 10.12111/j.mes.20200172

Source and time series of 239+240Pu in marine corals

More Information
  • Received Date: July 04, 2020
  • Revised Date: October 14, 2020
  • Available Online: February 15, 2022
  • The 10 time series of 239+240Pu specific activity and 240Pu/239Pu atom ratio in reef and atoll corals in the Pacific Ocean and Atlantic Ocean were analyzed and compared, at the same time discussed its source and its significance to the environment. The results showed that 239+240Pu in corals mainly came from global fallout and Pacific Proving Grounds (PPG) close-in fallout. As the difference growth environments between shore reefs and atolls, the time series of 239+240Pu in corals also showed different characteristics. Large-scale atmospheric nuclear weapons test between 1952 and 1958 in the Pacific Proving Grounds made close-in fallout or local input of Pu become the main source of available Pu for corals in seawater. The time series of 239+240Pu in corals have different time series patterns from that of global fallout Pu. So the time series of 239+240Pu specific activity in Pacific corals (the main peak time position corresponds to 1954) and in Atlantic corals (the main peak time position corresponds to 1964) have different patterns. Pu in corals maybe indicate the direction of seawater current, El Nio phenomena on a large spatial scale and the fluctuation period of lagoon seawater on a small spatial scale in ocean.

  • [1]
    NOSHKIN V E, WONG K M, EAGLE R J, et al. Transuranics and other radionuclides in Bikini Lagoon: concentration data retrieved from aged coral sections[J]. Limnology and Oceanography, 1975, 20(5): 729-742. doi: 10.4319/lo.1975.20.5.0729
    [2]
    DRUFFEL E R M, KING L L, BELASTOCK R A, et al. Growth rate of a deep-sea coral using 210Pb and other isotopes[J]. Geochimica et Cosmochimica Acta, 1990, 54(5): 1493-1499. doi: 10.1016/0016-7037(90)90174-J
    [3]
    余克服, 刘东生, 沈承德, 等. 雷州半岛全新世高温期珊瑚生长所揭示的环境突变事件[J]. 中国科学(D辑:地球科学), 2002, 32(2): 149–156.
    [4]
    林武辉, 余克服, 王英辉, 等. 珊瑚礁区沉积物的极低放射性水平特征与成因[J]. 科学通报, 2018, 63(21): 2173-2183.
    [5]
    张晓笛, 毕倩倩, 蔡炜颖, 等. 应用210Pb的南海黑角珊瑚定年[J]. 核化学与放射化学, 2015, 37(2): 120-128. doi: 10.7538/hhx.2015.37.02.0120
    [6]
    TOGGWEILER J R, TRUMBORE S. Bomb-test 90Sr in Pacific and Indian Ocean surface water as recorded by banded corals[J]. Earth and Planetary Science Letters, 1985, 74(4): 306-314. doi: 10.1016/S0012-821X(85)80002-9
    [7]
    BIDDULPH D L, BECK J W, BURR G S, et al. Two 60-year records of 129I from coral skeletons in the South Pacific Ocean[J]. Radioactivity in the Environment, 2006, 8: 592-598.
    [8]
    BAUTISTA VII A T, MATSUZAKI H, SIRINGAN F P. Historical record of nuclear activities from 129I in corals from the northern hemisphere (Philippines)[J]. Journal of Environmental Radioactivity, 2016, 164: 174-181. doi: 10.1016/j.jenvrad.2016.07.022
    [9]
    SAKAGUCHI A, NOMURA T, STEIER P, et al. Temporal and vertical distributions of anthropogenic 236U in the Japan Sea using a coral core and seawater samples[J]. Journal of Geophysical Research: Oceans, 2016, 121(1): 4-13. doi: 10.1002/2015JC011109
    [10]
    FROEHLICH M B, CHAN W Y, TIMS S G, et al. Time-resolved record of 236U and 239, 240Pu isotopes from a coral growing during the nuclear testing program at Enewetak Atoll (Marshall Islands)[J]. Journal of Environmental Radioactivity, 2016, 165: 197-205. doi: 10.1016/j.jenvrad.2016.09.015
    [11]
    FROEHLICH M B, TIMS S G, FALLON S J, et al. Nuclear weapons produced 236U, 239Pu and 240Pu archived in a Porites Lutea coral from Enewetak Atoll[J]. Journal of Environmental Radioactivity, 2017, 178/179: 349-353. doi: 10.1016/j.jenvrad.2017.05.009
    [12]
    MEECE D E, BENNINGER L K. The coprecipitation of Pu and other radionuclides with CaCO3[J]. Geochimica et Cosmochimica Acta, 1993, 57(7): 1447-1458. doi: 10.1016/0016-7037(93)90005-H
    [13]
    BENNINGER L K, DODGE R E. Fallout plutonium and natural radionuclides in annual bands of the coral Montastrea annularis, St. Croix, US Virgin Islands[J]. Geochimica et Cosmochimica Acta, 1986, 50(12): 2785-2797. doi: 10.1016/0016-7037(86)90227-9
    [14]
    PURDY C B, DRUFFEL E R M, LIVINGSTON H D. Anomalous levels of 90Sr and 239, 240Pu in Florida corals: Evidence of coastal processes[J]. Geochimica et Cosmochimica Acta, 1989, 53(6): 1401-1410. doi: 10.1016/0016-7037(89)90072-0
    [15]
    BUESSELER K O. The isotopic signature of fallout plutonium in the North Pacific[J]. Journal of Environmental Radioactivity, 1997, 36(1): 69-83. doi: 10.1016/S0265-931X(96)00071-9
    [16]
    LINDAHL P, ASAMI R, IRYU Y, et al. Sources of plutonium to the tropical Northwest Pacific Ocean (1943–1999) identified using a natural coral archive[J]. Geochimica et Cosmochimica Acta, 2011, 75(5): 1346-1356. doi: 10.1016/j.gca.2010.12.012
    [17]
    LINDAHL P, ANDERSEN M B, KEITH-ROACH M, et al. Spatial and temporal distribution of Pu in the Northwest Pacific Ocean using modern coral archives[J]. Environment International, 2012, 40: 196-201. doi: 10.1016/j.envint.2011.08.004
    [18]
    赵焕庭, 王丽荣, 袁家义. 南海诸岛珊瑚礁可持续发展[J]. 热带地理, 2016, 36(1): 55-65.
    [19]
    UNSCEAR. Sources and effects of ionizing radiation[C]//Report to the General Assembly, with Scientific Annexes. New York: United Nations, 2000.
    [20]
    KELLEY J M, BOND L A, BEASLEY T M. Global distribution of Pu isotopes and 237Np[J]. Science of the Total Environment, 1999, 237/238: 483-500. doi: 10.1016/S0048-9697(99)00160-6
    [21]
    SEABORG G T, PERLMAN M L. Search for Elements 94 and 93 in Nature. Presence of 94239 in Pitchblende1[J]. Journal of the American Chemical Society, 1948, 70(4): 1571-1573. doi: 10.1021/ja01184a083
    [22]
    PEPPARD D F, STUDIER M H, GERGEL M V, et al. Isolation of Microgram Quantities of Naturally-occurring Plutonium and Examination of its Isotopic Composition[J]. Journal of the American Chemical Society, 1951, 73(6): 2529-31. doi: 10.1021/ja01150a034
    [23]
    TAYLOR D M. Environmental plutonium-creation of the universe to twenty-first century mankind[J]. Radioactivity in the Environment, 2001, 1: 1-14.
    [24]
    IMAI T, SAKANOUE M. Content of plutonium, thorium and protactinium in sea water and recent coral in the North Pacific[J]. Journal of the Oceanographical Society of Japan, 1973, 29(2): 76-82.
    [25]
    MURAMATSU Y, HAMILTON T, UCHIDA S, et al. Measurement of 240Pu/239Pu isotopic ratios in soils from the Marshall Islands using ICP-MS[J]. Science of the Total Environment, 2001, 278(1/2/3): 151-159.
    [26]
    GUAN Y J, MAI J Y, WANG H J, et al. Plutonium isotopes and radionuclides in corals around Weizhou land in Beibu Gulf, China[J]. Applied Radiation and Isotopes, 2021, 176: 109873.

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